From Agricultural Residues to Sustainable Boards: Complex Network Analysis of Binderless Composites

Abstract

The transition toward sustainable panel technologies is driving intensive research on binderless boards and self-bonded lignocellulosic composites. Particleboard, an engineered wood composite made by hot pressing wood particles with synthetic adhesives, is among the most widely produced wood-based panels due to cost-effectiveness and versatility. However, pressure on forest-derived raw materials and concern over formaldehyde emissions are accelerating the search for renewable resources and greener routes. Residues and underutilized materials from agro-industrial, food, and forestry sectors (such as cereal straws, sugarcane bagasse, brewer’s spent grain, and fruit-processing by-products) offer a sustainable alternative, enabling waste valorization, lowering environmental burdens, and supporting circular bioeconomy models. Binderless boards, produced without adhesives, exploit natural bonding among lignocellulosic components, including lignin softening, thermoplasticization, and covalent crosslinking during hot pressing. This review adopts a complex network approach to systematically map and analyze the scientific landscape of binderless board production. Using citation-based networks from curated seed papers and their first- and second-degree neighbors, we identify thematic clusters, with cluster “A” as the research core. The examination of this cluster, complemented by word-cloud analysis of titles and abstracts, highlights prevalent raw materials and key research lines, like rawmaterial sources and lignocellulosic composition, processing parameters, and pretreatment strategies. Based on these findings, brewer’s spent grain is selected as a representative case study for cost analysis. This approach synthesizes the state of the art and reveals emerging directions, research gaps, and influential works, providing a data-driven foundation for advancing self-bonded lignocellulosic composites.