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dc.contributor.author
Fornero, Esteban Luis
dc.contributor.author
Giombi, Jose Luis
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Chiavassa, Dante Luis
dc.contributor.author
Bonivardi, Adrian Lionel
dc.contributor.author
Baltanas, Miguel Angel
dc.date.available
2016-12-22T18:48:49Z
dc.date.issued
2015-01
dc.identifier.citation
Fornero, Esteban Luis; Giombi, Jose Luis; Chiavassa, Dante Luis; Bonivardi, Adrian Lionel; Baltanas, Miguel Angel; A versatile Carberry-type microcatalytic reactor for transient and/or continuous flow operation at atmospheric or medium pressure; Elsevier Science Sa; Chemical Engineering Journal; 264; 1-2015; 664-671
dc.identifier.issn
1385-8947
dc.identifier.uri
http://hdl.handle.net/11336/9952
dc.description.abstract
A novel catalytic reaction device featuring a Carberry-type well-mixed microreactor built inside a medium pressure leak valve is presented. The complete reaction system allows a broad range of kinetic reaction engineering and heterogeneous catalysis studies for both batch (transient) and continuous operation. Carefully controlled temperature (± 0.2 K) and pressure (up to 3 MPa) conditions can be achieved. The continuous sampling of the reacting mixture permits instantaneous evaluation of the gas phase composition. The device performance was validated by comparing methanol synthesis reaction rates for H2/CO2 mixtures obtained under transient conditions using this catalytic microreactor with steady-state kinetic rate expressions obtained using a conventional plug-flow microreactor employing the same Pd-GaOx/SiO2 catalyst. Excellent agreement was found. The reaction was also studied using a more active commercial methanol synthesis catalyst to assess the impact of heat and mass transfer resistances. For the full range of process conditions that was tested, the microreactor operated well under the kinetic regime.
dc.format
application/pdf
dc.language.iso
eng
dc.publisher
Elsevier Science Sa
dc.rights
info:eu-repo/semantics/openAccess
dc.rights.uri
https://creativecommons.org/licenses/by-nc-sa/2.5/ar/
dc.subject
Microcatalytic Reactor
dc.subject
Carberry-Type
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Transient Experiments
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Kinetic Regime
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Ingeniería de Procesos Químicos
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Ingeniería Química
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INGENIERÍAS Y TECNOLOGÍAS
dc.title
A versatile Carberry-type microcatalytic reactor for transient and/or continuous flow operation at atmospheric or medium pressure
dc.type
info:eu-repo/semantics/article
dc.type
info:ar-repo/semantics/artículo
dc.type
info:eu-repo/semantics/publishedVersion
dc.date.updated
2016-12-16T14:26:58Z
dc.journal.volume
264
dc.journal.pagination
664-671
dc.journal.pais
Países Bajos
dc.journal.ciudad
Amsterdam
dc.description.fil
Fil: Fornero, Esteban Luis. Consejo Nacional de Investigaciones Científicas y Técnicas. Centro Científico Tecnológico Santa Fe. Instituto de Desarrollo Tecnológico Para la Industria Química (i); Argentina
dc.description.fil
Fil: Giombi, Jose Luis. Consejo Nacional de Investigaciones Científicas y Técnicas. Centro Científico Tecnológico Santa Fe. Instituto de Desarrollo Tecnológico Para la Industria Química (i); Argentina
dc.description.fil
Fil: Chiavassa, Dante Luis. Consejo Nacional de Investigaciones Científicas y Técnicas. Centro Científico Tecnológico Santa Fe. Instituto de Desarrollo Tecnológico Para la Industria Química (i); Argentina
dc.description.fil
Fil: Bonivardi, Adrian Lionel. Consejo Nacional de Investigaciones Científicas y Técnicas. Centro Científico Tecnológico Santa Fe. Instituto de Desarrollo Tecnológico Para la Industria Química (i); Argentina
dc.description.fil
Fil: Baltanas, Miguel Angel. Consejo Nacional de Investigaciones Científicas y Técnicas. Centro Científico Tecnológico Santa Fe. Instituto de Desarrollo Tecnológico Para la Industria Química (i); Argentina
dc.journal.title
Chemical Engineering Journal
dc.relation.alternativeid
info:eu-repo/semantics/altIdentifier/url/http://www.sciencedirect.com/science/article/pii/S1385894714015745
dc.relation.alternativeid
info:eu-repo/semantics/altIdentifier/doi/http://dx.doi.org/10.1016/j.cej.2014.11.106
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