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dc.contributor.author
Appignanesi, Gustavo Adrian  
dc.contributor.author
Alarcon, Laureano Martin  
dc.contributor.author
Rodriguez Fris, Jorge Ariel  
dc.contributor.author
Frechero, Marisa Alejandra  
dc.contributor.author
Montani, Rosana A.  
dc.date.available
2020-01-09T20:47:44Z  
dc.date.issued
2005-04  
dc.identifier.citation
Appignanesi, Gustavo Adrian; Alarcon, Laureano Martin; Rodriguez Fris, Jorge Ariel; Frechero, Marisa Alejandra; Montani, Rosana A.; Activated dynamics and timescale separation within the landscape paradigm: Signature of complexity, diversity and glassiness; Elsevier Science; Biophysical Chemistry; 115; 2-3 SPEC. ISS.; 4-2005; 129-134  
dc.identifier.issn
0301-4622  
dc.identifier.uri
http://hdl.handle.net/11336/94248  
dc.description.abstract
The landscape paradigm has become a widespread picture within the realm of complex systems. Complex systems include a great variety of systems, ranging from glasses to biopolymers, which display a common dynamical behavior. Within this framework, the dynamics of a such a system can be envisioned as the search it performs on its (potential energy) landscape. This approach rests on the belief that the relaxation behavior depends only on generic features, irrespective of specific details and lies on the validity of a timescale separation scenario computationally corroborated but not properly validated yet form first principles. In this work we shall show that the prevalence of activated dynamics over other kinds of mechanisms determines the emergence of complex dynamical behavior. Thus, complexity and diversity are not intrinsic properties of a system but depend on the kind of exploration of the landscape. We shall focus mainly on an ample generic context (complex hierarchical systems which have been used as models of glasses, spin glasses and biopolymers) and a specific one (model glass formers). For the last case we shall be able to reveal (in mechanistic terms) the microscopic rationale for the occurrence of timescale separation. Furthermore, we shall explore the connections between these two up to now mostly unrelated contexts and the relation to a variational principle, and we shall reveal the conditions for the applicability of the landscape approach.  
dc.format
application/pdf  
dc.language.iso
eng  
dc.publisher
Elsevier Science  
dc.rights
info:eu-repo/semantics/openAccess  
dc.rights.uri
https://creativecommons.org/licenses/by-nc-nd/2.5/ar/  
dc.subject
ACTIVATED DYNAMICS  
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BIOPOLYMER FOLDING  
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COMPLEX SYSTEMS  
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GLASSY SYSTEMS  
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HIERARCHICAL SYSTEMS  
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MOLECULAR DYNAMICS  
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RELAXATION  
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ULTRAMETRIC SPACES  
dc.subject.classification
Físico-Química, Ciencia de los Polímeros, Electroquímica  
dc.subject.classification
Ciencias Químicas  
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CIENCIAS NATURALES Y EXACTAS  
dc.title
Activated dynamics and timescale separation within the landscape paradigm: Signature of complexity, diversity and glassiness  
dc.type
info:eu-repo/semantics/article  
dc.type
info:ar-repo/semantics/artículo  
dc.type
info:eu-repo/semantics/publishedVersion  
dc.date.updated
2019-11-27T14:52:06Z  
dc.journal.volume
115  
dc.journal.number
2-3 SPEC. ISS.  
dc.journal.pagination
129-134  
dc.journal.pais
Países Bajos  
dc.journal.ciudad
Amsterdam  
dc.description.fil
Fil: Appignanesi, Gustavo Adrian. Consejo Nacional de Investigaciones Científicas y Técnicas. Centro Científico Tecnológico Conicet - Bahía Blanca. Instituto de Química del Sur. Universidad Nacional del Sur. Departamento de Química. Instituto de Química del Sur; Argentina  
dc.description.fil
Fil: Alarcon, Laureano Martin. Consejo Nacional de Investigaciones Científicas y Técnicas. Centro Científico Tecnológico Conicet - Bahía Blanca. Instituto de Química del Sur. Universidad Nacional del Sur. Departamento de Química. Instituto de Química del Sur; Argentina  
dc.description.fil
Fil: Rodriguez Fris, Jorge Ariel. Consejo Nacional de Investigaciones Científicas y Técnicas. Centro Científico Tecnológico Conicet - Bahía Blanca. Instituto de Química del Sur. Universidad Nacional del Sur. Departamento de Química. Instituto de Química del Sur; Argentina  
dc.description.fil
Fil: Frechero, Marisa Alejandra. Consejo Nacional de Investigaciones Científicas y Técnicas. Centro Científico Tecnológico Conicet - Bahía Blanca. Instituto de Química del Sur. Universidad Nacional del Sur. Departamento de Química. Instituto de Química del Sur; Argentina  
dc.description.fil
Fil: Montani, Rosana A.. Universidad Nacional del Sur. Departamento de Química; Argentina  
dc.journal.title
Biophysical Chemistry  
dc.relation.alternativeid
info:eu-repo/semantics/altIdentifier/url/https://www.sciencedirect.com/science/article/abs/pii/S0301462204003564  
dc.relation.alternativeid
info:eu-repo/semantics/altIdentifier/doi/http://dx.doi.org/10.1016/j.bpc.2004.12.017