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dc.contributor.author
Carbajal Ramos, Ines Alejandra
dc.contributor.author
Andrade Gamboa, Julio José
dc.contributor.author
Gennari, Fabiana Cristina
dc.date.available
2016-12-07T16:22:20Z
dc.date.issued
2013-11
dc.identifier.citation
Carbajal Ramos, Ines Alejandra; Andrade Gamboa, Julio José; Gennari, Fabiana Cristina; Nanostructured Ce1-xZrxO2 Solid Solutions Produced by Mechanochemical Processing; Elsevier Science Sa; Materials Chemistry And Physics; 137; 3; 11-2013; 1073-1080
dc.identifier.issn
0254-0584
dc.identifier.uri
http://hdl.handle.net/11336/8986
dc.description.abstract
The nanostructured Ce1xZrxO2solid solutions (x0.2) have been successfully synthesized from CeCl3-ZrCl4-NaOH mixtures by mechanochemical processing as a gradual transformation, involvingin-situ CeO2and amorphous ZrO2formation as intermediates. Solid solutions type-Ce1xZrxO2along with NaCl as diluent were obtained at different milling times, with afinal composition of Ce0.8Zr0.2O2after 5 h and 15 h under high and low energetic milling conditions, respectively. The NaCl formed during the mechanochemical reaction, which is eliminated by washing after calcination of the as-milled sample, allows to obtain a Ce0.8Zr0.2O2solid solution with high surface area and nanometric grains. The nanostructured Ce0.8Zr0.2O2solid solution shows good thermal stability after prolonged heating at 600 C. However, the addition of an extra amount of diluent during mechanochemical reaction evidences a detrimental effect, avoiding the formation of solid solution or deteriorating the textural/microstructuctural characteristics of the obtained Ce1xZrxO2solid solution. Removal of NaCl previous to calcination improves notably the textural/microstructural characteristics of the Ce0.8Zr0.2O2solid solution.
dc.format
application/pdf
dc.language.iso
eng
dc.publisher
Elsevier Science Sa
dc.rights
info:eu-repo/semantics/openAccess
dc.rights.uri
https://creativecommons.org/licenses/by-nc-nd/2.5/ar/
dc.subject
Oxides
dc.subject
Microstructure
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Powder Diffraction
dc.subject
Nanostructure
dc.subject.classification
Ingeniería del Petróleo, Energía y Combustibles
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Ingeniería del Medio Ambiente
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INGENIERÍAS Y TECNOLOGÍAS
dc.title
Nanostructured Ce1-xZrxO2 Solid Solutions Produced by Mechanochemical Processing
dc.type
info:eu-repo/semantics/article
dc.type
info:ar-repo/semantics/artículo
dc.type
info:eu-repo/semantics/publishedVersion
dc.date.updated
2016-12-06T16:31:49Z
dc.journal.volume
137
dc.journal.number
3
dc.journal.pagination
1073-1080
dc.journal.pais
Países Bajos
dc.journal.ciudad
Ámsterdam
dc.description.fil
Fil: Carbajal Ramos, Ines Alejandra. Comisión Nacional de Energía Atómica. Gerencia del Area de Energía Nuclear. Instituto Balseiro; Argentina. Comision Nacional de Energia Atomica. Gerencia del Area de Investigaciones y Aplicaciones no Nucleares. Gerencia de Fisica (CAB); Argentina. Consejo Nacional de Investigaciones Científicas y Técnicas. Centro Científico Tecnológico Conicet - Patagonia Norte; Argentina
dc.description.fil
Fil: Andrade Gamboa, Julio José. Comisión Nacional de Energía Atómica. Gerencia del Area de Energía Nuclear. Instituto Balseiro; Argentina. Comision Nacional de Energia Atomica. Gerencia del Area de Investigaciones y Aplicaciones no Nucleares. Gerencia de Fisica (CAB); Argentina
dc.description.fil
Fil: Gennari, Fabiana Cristina. Consejo Nacional de Investigaciones Científicas y Técnicas. Centro Científico Tecnológico Conicet - Patagonia Norte; Argentina. Comisión Nacional de Energía Atómica. Gerencia del Area de Energía Nuclear. Instituto Balseiro; Argentina. Comision Nacional de Energia Atomica. Gerencia del Area de Investigaciones y Aplicaciones no Nucleares. Gerencia de Fisica (CAB); Argentina
dc.journal.title
Materials Chemistry And Physics
dc.relation.alternativeid
info:eu-repo/semantics/altIdentifier/url/http://www.sciencedirect.com/science/article/pii/S0254058412009820
dc.relation.alternativeid
info:eu-repo/semantics/altIdentifier/doi/http://dx.doi.org/10.1016/j.matchemphys.2012.11.039
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