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dc.contributor.author
Lopez, Eduardo  
dc.contributor.author
Gepert, Vanessa  
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Gritsch, Achim  
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Nieken, Ulrich  
dc.contributor.author
Eigenberger, Gerhart  
dc.date.available
2019-05-27T16:01:05Z  
dc.date.issued
2012-03-28  
dc.identifier.citation
Lopez, Eduardo; Gepert, Vanessa; Gritsch, Achim; Nieken, Ulrich; Eigenberger, Gerhart; Ethanol steam reforming thermally coupled with fuel combustion in a parallel plate reactor; American Chemical Society; Industrial & Engineering Chemical Research; 51; 11; 28-3-2012; 4143-4151  
dc.identifier.issn
0888-5885  
dc.identifier.uri
http://hdl.handle.net/11336/77176  
dc.description.abstract
This contribution reports experimental studies of ethanol steam reforming for the production of a hydrogen-rich reformate for fuel cells. A Pd-based catalyst, coated on corrugated metallic structures, was used. Axial concentration profiles for all components present in the system were measured in a kinetic reactor under isothermal conditions for different temperatures, flow rates, and steam-to-carbon ratios. Appropriate activity and hydrogen selectivity were achieved for this catalytic system at 650 °C, with complete ethanol conversion (no acetaldehyde), ca. 5% carbon monoxide and 1% methane as byproducts. For reactor modeling in an appropriate range of operating conditions, a simple global kinetics model is proposed; the correspondent parameters were fitted to the experimental data. Thermal coupling between ethanol steam reforming and hydrogen combustion was experimentally studied for subsequent implementation in a parallel-plate reactor, preferably in a so-called folded plate reactor. A single unit of this reactor, consisting of one combustion channel in between two halves of reforming channels was selected for the experimental proof-of-concept. The influence of different operating variables (ethanol load, feed distribution of the combustion fuel along the channel length, operation temperature, and steam-to-carbon ratio) on the reactor performance and the thermal coupling pattern will be discussed.  
dc.format
application/pdf  
dc.language.iso
eng  
dc.publisher
American Chemical Society  
dc.rights
info:eu-repo/semantics/openAccess  
dc.rights.uri
https://creativecommons.org/licenses/by-nc-sa/2.5/ar/  
dc.subject
Ethanol  
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Steam Reforming  
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Plate Reactor  
dc.subject.classification
Otras Ingeniería Química  
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Ingeniería Química  
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INGENIERÍAS Y TECNOLOGÍAS  
dc.title
Ethanol steam reforming thermally coupled with fuel combustion in a parallel plate reactor  
dc.type
info:eu-repo/semantics/article  
dc.type
info:ar-repo/semantics/artículo  
dc.type
info:eu-repo/semantics/publishedVersion  
dc.date.updated
2019-05-14T17:40:00Z  
dc.journal.volume
51  
dc.journal.number
11  
dc.journal.pagination
4143-4151  
dc.journal.pais
Estados Unidos  
dc.journal.ciudad
Washington DC  
dc.description.fil
Fil: Lopez, Eduardo. Consejo Nacional de Investigaciones Científicas y Técnicas. Centro Científico Tecnológico Conicet - Bahía Blanca. Planta Piloto de Ingeniería Química. Universidad Nacional del Sur. Planta Piloto de Ingeniería Química; Argentina. University of Stuttgart; Alemania  
dc.description.fil
Fil: Gepert, Vanessa. University of Stuttgart; Alemania  
dc.description.fil
Fil: Gritsch, Achim. University of Stuttgart; Alemania  
dc.description.fil
Fil: Nieken, Ulrich. University of Stuttgart; Alemania  
dc.description.fil
Fil: Eigenberger, Gerhart. University of Stuttgart; Alemania  
dc.journal.title
Industrial & Engineering Chemical Research  
dc.relation.alternativeid
info:eu-repo/semantics/altIdentifier/url/https://pubs.acs.org/doi/pdf/10.1021/ie202364y  
dc.relation.alternativeid
info:eu-repo/semantics/altIdentifier/doi/http://dx.doi.org/10.1021/ie202364y