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dc.contributor.author
Brinks, Daan
dc.contributor.author
Hildner, Richard
dc.contributor.author
Stefani, Fernando Daniel
dc.contributor.author
Van Hulst, Niek F.
dc.date.available
2019-01-29T21:27:42Z
dc.date.issued
2011-12
dc.identifier.citation
Brinks, Daan; Hildner, Richard; Stefani, Fernando Daniel; Van Hulst, Niek F.; Beating spatio-temporal coupling: Implications for pulse shaping and coherent control experiments; Optical Society of America; Optics Express; 19; 27; 12-2011; 26486-26499
dc.identifier.issn
1094-4087
dc.identifier.uri
http://hdl.handle.net/11336/68943
dc.description.abstract
Diffraction of finite sized laser beams imposes a limit on the control that can be exerted over ultrafast pulses. This limit manifests as spatio-temporal coupling induced in standard implementations of pulse shaping schemes. We demonstrate the influence this has on coherent control experiments that depend on finite excitation, sample, and detection volumes. Based on solutions used in pulse stretching experiments, we introduce a double-pass scheme that reduces the errors produced through spatio-temporal coupling by at least one order of magnitude. Finally, employing single molecules as nanoscale probes, we prove that such a double pass scheme is capable of artifact-free pulse shaping at dimensions two orders of magnitude smaller than the diffraction limit.
dc.format
application/pdf
dc.language.iso
eng
dc.publisher
Optical Society of America
dc.rights
info:eu-repo/semantics/openAccess
dc.rights.uri
https://creativecommons.org/licenses/by-nc-sa/2.5/ar/
dc.subject
Ultrafast Spectroscopy
dc.subject
Pulse Shaper
dc.subject.classification
Óptica
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Ciencias Físicas
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CIENCIAS NATURALES Y EXACTAS
dc.title
Beating spatio-temporal coupling: Implications for pulse shaping and coherent control experiments
dc.type
info:eu-repo/semantics/article
dc.type
info:ar-repo/semantics/artículo
dc.type
info:eu-repo/semantics/publishedVersion
dc.date.updated
2019-01-29T18:06:20Z
dc.journal.volume
19
dc.journal.number
27
dc.journal.pagination
26486-26499
dc.journal.pais
Estados Unidos
dc.description.fil
Fil: Brinks, Daan. Institut de Ciencies Fotoniques; España
dc.description.fil
Fil: Hildner, Richard. Institut de Ciencies Fotoniques; España. University of Bayreuth; Alemania
dc.description.fil
Fil: Stefani, Fernando Daniel. Institut de Ciencies Fotoniques; España. Consejo Nacional de Investigaciones Científicas y Técnicas. Oficina de Coordinación Administrativa Parque Centenario. Centro de Investigaciones en Bionanociencias "Elizabeth Jares Erijman"; Argentina
dc.description.fil
Fil: Van Hulst, Niek F.. Universidad de Barcelona. Institució Catalana de Recerca i Estudis Avançats; España. Institut de Ciencies Fotoniques; España
dc.journal.title
Optics Express
dc.relation.alternativeid
info:eu-repo/semantics/altIdentifier/url/https://www.osapublishing.org/oe/abstract.cfm?uri=oe-19-27-26486
dc.relation.alternativeid
info:eu-repo/semantics/altIdentifier/doi/http://dx.doi.org/10.1364/OE.19.026486
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