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dc.contributor.author
Fischereder, Achim
dc.contributor.author
Martinez Ricci, Maria Luz
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Wolosiuk, Alejandro
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Haas, Wernfried
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Hofer, Ferdinand
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Trimmel, Gregor
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Soler Illia, Galo Juan de Avila Arturo
dc.date.available
2019-01-09T20:12:33Z
dc.date.issued
2012-05
dc.identifier.citation
Fischereder, Achim; Martinez Ricci, Maria Luz; Wolosiuk, Alejandro; Haas, Wernfried; Hofer, Ferdinand; et al.; Mesoporous ZnS thin films prepared by a nanocasting route; American Chemical Society; Chemistry Of Materials; 24; 10; 5-2012; 1837-1845
dc.identifier.issn
0897-4756
dc.identifier.uri
http://hdl.handle.net/11336/67851
dc.description.abstract
Mesoporous metal chalcogenides (e.g., ZnS, CuS, and derived mixed sulfide or selenides) show an extremely high potential in technological areas like catalysis, sensors, environmental protection, and photovoltaics. Although chemical bath deposition methods allow obtaining stable and porous metal chalcogenide films under mild and simple conditions, the reproducible preparation of highly ordered mesoporous sulfide thin films has been challenging so far. Herein, we present a simple and efficient synthetic method to prepare ZnS mesoporous thin films using a combination of a nanocasting approach and a successive ionic layer adsorption and reaction (SILAR) process for the infiltration. A mesoporous silica thin film, prepared by evaporation induced self-assembly (EISA), serves as the hard exotemplate for the formation of the mesostructured zinc sulfide. After selective etching of the silica framework, a stable and porous ZnS thin film is obtained, which replicates the pore structure of the hard template. A thorough combination of characterization techniques is used to assess the exotemplating process as well as the template removal. © 2012 American Chemical Society.
dc.format
application/pdf
dc.language.iso
eng
dc.publisher
American Chemical Society
dc.rights
info:eu-repo/semantics/restrictedAccess
dc.rights.uri
https://creativecommons.org/licenses/by-nc-sa/2.5/ar/
dc.subject
Mesoporous Film
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Nanocasting
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Silar
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Zinc Sulfide
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Nano-materiales
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Nanotecnología
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INGENIERÍAS Y TECNOLOGÍAS
dc.title
Mesoporous ZnS thin films prepared by a nanocasting route
dc.type
info:eu-repo/semantics/article
dc.type
info:ar-repo/semantics/artículo
dc.type
info:eu-repo/semantics/publishedVersion
dc.date.updated
2019-01-02T19:32:19Z
dc.journal.volume
24
dc.journal.number
10
dc.journal.pagination
1837-1845
dc.journal.pais
Estados Unidos
dc.journal.ciudad
Washington
dc.description.fil
Fil: Fischereder, Achim. Graz University of Technology; Austria
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Fil: Martinez Ricci, Maria Luz. Consejo Nacional de Investigaciones Científicas y Técnicas; Argentina. Comisión Nacional de Energía Atómica. Centro Atómico Constituyentes; Argentina. Universidad de Buenos Aires. Facultad de Ciencias Exactas y Naturales. Departamento de Química Inorgánica, Analítica y Química Física; Argentina
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Fil: Wolosiuk, Alejandro. Consejo Nacional de Investigaciones Científicas y Técnicas; Argentina. Comisión Nacional de Energía Atómica. Centro Atómico Constituyentes; Argentina
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Fil: Haas, Wernfried. Graz University of Technology; Austria
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Fil: Hofer, Ferdinand. Graz University of Technology; Austria
dc.description.fil
Fil: Trimmel, Gregor. Graz University of Technology; Austria
dc.description.fil
Fil: Soler Illia, Galo Juan de Avila Arturo. Consejo Nacional de Investigaciones Científicas y Técnicas; Argentina. Comisión Nacional de Energía Atómica. Centro Atómico Constituyentes; Argentina
dc.journal.title
Chemistry Of Materials
dc.relation.alternativeid
info:eu-repo/semantics/altIdentifier/url/https://pubs.acs.org/doi/abs/10.1021/cm300395m
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info:eu-repo/semantics/altIdentifier/doi/https://dx.doi.org/10.1021/cm300395m