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dc.contributor.author
Dieuzeide, María Laura
dc.contributor.author
Laborde, Miguel Ángel
dc.contributor.author
Amadeo, Norma Elvira
dc.contributor.author
Cannilla, C.
dc.contributor.author
Bonura, G.
dc.contributor.author
Frusteri, F.
dc.date.available
2018-09-19T17:59:09Z
dc.date.issued
2016-01
dc.identifier.citation
Dieuzeide, María Laura; Laborde, Miguel Ángel; Amadeo, Norma Elvira; Cannilla, C.; Bonura, G.; et al.; Hydrogen production by glycerol steam reforming: How Mg doping affects the catalytic behaviour of Ni/Al2O3 catalysts; Pergamon-Elsevier Science Ltd; International Journal of Hydrogen Energy; 41; 1; 1-2016; 157-166
dc.identifier.issn
0360-3199
dc.identifier.uri
http://hdl.handle.net/11336/60253
dc.description.abstract
Glycerol steam reforming, using Mg doped Ni/Al2O3 catalysts, was investigated with the aim to efficiently produce hydrogen. Catalyst containing different Mg loading were prepared by impregnation method maintaining constant the Ni loading (10 wt.%). Catalytic experiments were performed in fixed bed reactor operated at 500 and 600 °C. Characterization results revealed that Mg, further to infer a basic character to the carrier, promotes the Ni dispersion. In addition to observe that the catalytic activity was mainly dependent upon the Ni dispersion, the amount and morphology of coke formed during reaction was affected by Mg loading. In particular, the addition of 3wt% of Mg contributes to reduce the coke formation rate while a subsequent addition of Mg up to 10wt%, does not significantly affect neither the catalytic activity nor the carbon formation. By operating at 600 °C and with H2O/Gly ratio of 6, low amount of coke, mainly of filamentous nature, was formed. The size and structure of carbon filaments changed as a function of Ni particle size and Mg loading.
dc.format
application/pdf
dc.language.iso
eng
dc.publisher
Pergamon-Elsevier Science Ltd
dc.rights
info:eu-repo/semantics/restrictedAccess
dc.rights.uri
https://creativecommons.org/licenses/by-nc-nd/2.5/ar/
dc.subject
Glycerol Steam Reforming
dc.subject
Hydrogen Production
dc.subject
Ni-Mg Catalysts
dc.subject.classification
Otras Ingeniería Química
dc.subject.classification
Ingeniería Química
dc.subject.classification
INGENIERÍAS Y TECNOLOGÍAS
dc.title
Hydrogen production by glycerol steam reforming: How Mg doping affects the catalytic behaviour of Ni/Al2O3 catalysts
dc.type
info:eu-repo/semantics/article
dc.type
info:ar-repo/semantics/artículo
dc.type
info:eu-repo/semantics/publishedVersion
dc.date.updated
2018-09-18T13:17:27Z
dc.journal.volume
41
dc.journal.number
1
dc.journal.pagination
157-166
dc.journal.pais
Estados Unidos
dc.description.fil
Fil: Dieuzeide, María Laura. Consejo Nacional de Investigaciones Científicas y Técnicas. Oficina de Coordinación Administrativa Ciudad Universitaria. Instituto de Tecnologías del Hidrogeno y Energias Sostenibles. Universidad de Buenos Aires. Facultad de Ingeniería. Instituto de Tecnologías del Hidrogeno y Energias Sostenibles; Argentina
dc.description.fil
Fil: Laborde, Miguel Ángel. Consejo Nacional de Investigaciones Científicas y Técnicas. Oficina de Coordinación Administrativa Ciudad Universitaria. Instituto de Tecnologías del Hidrogeno y Energias Sostenibles. Universidad de Buenos Aires. Facultad de Ingeniería. Instituto de Tecnologías del Hidrogeno y Energias Sostenibles; Argentina
dc.description.fil
Fil: Amadeo, Norma Elvira. Consejo Nacional de Investigaciones Científicas y Técnicas. Oficina de Coordinación Administrativa Ciudad Universitaria. Instituto de Tecnologías del Hidrogeno y Energias Sostenibles. Universidad de Buenos Aires. Facultad de Ingeniería. Instituto de Tecnologías del Hidrogeno y Energias Sostenibles; Argentina
dc.description.fil
Fil: Cannilla, C.. Consiglio Nazionale delle Ricerche; Italia
dc.description.fil
Fil: Bonura, G.. Consiglio Nazionale delle Ricerche; Italia
dc.description.fil
Fil: Frusteri, F.. Consiglio Nazionale delle Ricerche; Italia
dc.journal.title
International Journal of Hydrogen Energy
dc.relation.alternativeid
info:eu-repo/semantics/altIdentifier/doi/http://dx.doi.org/10.1016/j.ijhydene.2015.12.009
dc.relation.alternativeid
info:eu-repo/semantics/altIdentifier/url/https://www.sciencedirect.com/science/article/pii/S0360319915027536


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