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dc.contributor.author
Catalano, Paolo Nicolás
dc.contributor.author
Wolosiuk, Alejandro
dc.contributor.author
Soler Illia, Galo Juan de Avila Arturo
dc.contributor.author
Bellino, Martin Gonzalo
dc.date.available
2018-03-09T20:06:28Z
dc.date.issued
2015-12
dc.identifier.citation
Catalano, Paolo Nicolás; Wolosiuk, Alejandro; Soler Illia, Galo Juan de Avila Arturo; Bellino, Martin Gonzalo; Wired Enzymes in mesoporous materials: A benchmark for fabricating biofuel cells; Elsevier Science Sa; Bioelectrochemistry; 106; 12-2015; 14-21
dc.identifier.issn
1567-5394
dc.identifier.uri
http://hdl.handle.net/11336/38471
dc.description.abstract
Evolution of fuel cells using metallic inorganic catalysts has led to the development of biofuel cells with potential applications in implantable devices. However, the main disadvantages in real world applications of enzymatic biofuel cells are short lifetime and low power density. Many efforts have been devoted to immobilize redox enzymes on surfaces to allow efficient electrical communication with electrodes and to provide an adequate habitat for biochemical activity. In this context, nanocavities of mesoporous materials offer a tailored environment for protein immobilization. Mesostructured platforms with high surface area and stability have been developed to enhance mass transport, charge transfer from biocatalysts to electrodes and enzyme stability, leading to biofuel cells with improved power density (up to 602 μW cm− 2 at physiological conditions) and overall performance (high stability after 30 h of continuous operation and after 10 days of storage). This review discusses recent developments using mesoporous materials as novel platforms for effective electronic charge transfer in the context of current and emerging technologies in enzymatic fuel cell research, emphasizing their practical implications and potential improvements leading to a major impact on medical science and portable electronics.
dc.format
application/pdf
dc.language.iso
eng
dc.publisher
Elsevier Science Sa
dc.rights
info:eu-repo/semantics/openAccess
dc.rights.uri
https://creativecommons.org/licenses/by-nc-nd/2.5/ar/
dc.subject
Mesoporous Materials
dc.subject
Enzymatic Biofuel Cells
dc.subject
Enzyme Wiring
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Otras Ciencias Químicas
dc.subject.classification
Ciencias Químicas
dc.subject.classification
CIENCIAS NATURALES Y EXACTAS
dc.title
Wired Enzymes in mesoporous materials: A benchmark for fabricating biofuel cells
dc.type
info:eu-repo/semantics/article
dc.type
info:ar-repo/semantics/artículo
dc.type
info:eu-repo/semantics/publishedVersion
dc.date.updated
2018-03-09T18:58:06Z
dc.journal.volume
106
dc.journal.pagination
14-21
dc.journal.pais
Países Bajos
dc.journal.ciudad
Amsterdam
dc.description.fil
Fil: Catalano, Paolo Nicolás. Comisión Nacional de Energía Atómica; Argentina. Consejo Nacional de Investigaciones Científicas y Técnicas; Argentina
dc.description.fil
Fil: Wolosiuk, Alejandro. Comisión Nacional de Energía Atómica. Centro Atómico Constituyentes; Argentina. Consejo Nacional de Investigaciones Científicas y Técnicas; Argentina
dc.description.fil
Fil: Soler Illia, Galo Juan de Avila Arturo. Comisión Nacional de Energía Atómica. Centro Atómico Constituyentes; Argentina. Consejo Nacional de Investigaciones Científicas y Técnicas; Argentina
dc.description.fil
Fil: Bellino, Martin Gonzalo. Comisión Nacional de Energía Atómica. Centro Atómico Constituyentes; Argentina. Consejo Nacional de Investigaciones Científicas y Técnicas; Argentina
dc.journal.title
Bioelectrochemistry
dc.relation.alternativeid
info:eu-repo/semantics/altIdentifier/doi/http://dx.doi.org/10.1016/j.bioelechem.2015.06.006
dc.relation.alternativeid
info:eu-repo/semantics/altIdentifier/url/https://www.sciencedirect.com/science/article/pii/S1567539415000833
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