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dc.contributor.author
Hojamberdiev, Mirabbos  
dc.contributor.author
Vargas Balda, Ronald Eduardo  
dc.contributor.author
Zhang, Fuxiang  
dc.contributor.author
Teshima, Katsuya  
dc.contributor.author
Lerch, Martin  
dc.date.available
2024-12-13T12:29:32Z  
dc.date.issued
2023-10  
dc.identifier.citation
Hojamberdiev, Mirabbos; Vargas Balda, Ronald Eduardo; Zhang, Fuxiang; Teshima, Katsuya; Lerch, Martin; Perovskite BaTaO 2 N: From Materials Synthesis to Solar Water Splitting; Wiley; Advanced Science; 10; 33; 10-2023; 1-47  
dc.identifier.issn
2198-3844  
dc.identifier.uri
http://hdl.handle.net/11336/250427  
dc.description.abstract
Barium tantalum oxynitride (BaTaO2N), as a member of an emerging class of perovskite oxynitrides, is regarded as a promising inorganic material for solar water splitting because of its small band gap, visible light absorption, and suitable band edge potentials for overall water splitting in the absence of an external bias. However, BaTaO2N still exhibits poor water-splitting performance that is susceptible to its synthetic history, surface states, recombination process, and instability. This review provides a comprehensive summary of previous progress, current advances, existing challenges, and future perspectives of BaTaO2N for solar water splitting. A particular emphasis is given to highlighting the principles of photoelectrochemical (PEC) water splitting, classic and emerging photocatalysts for oxygen evolution reactions, and the crystal and electronic structures, dielectric, ferroelectric, and piezoelectric properties, synthesis routes, and thin-film fabrication of BaTaO2N. Various strategies to achieve enhanced water-splitting performance of BaTaO2N, such as reducing the surface and bulk defect density, engineering the crystal facets, tailoring the particle morphology, size, and porosity, cation doping, creating the solid solutions, forming the heterostructures and heterojunctions, designing the photoelectrochemical cells, and loading suitable cocatalysts are discussed. Also, the avenues for further investigation and the prospects of using BaTaO2N in solar water splitting are presented.  
dc.format
application/pdf  
dc.language.iso
eng  
dc.publisher
Wiley  
dc.rights
info:eu-repo/semantics/openAccess  
dc.rights.uri
https://creativecommons.org/licenses/by/2.5/ar/  
dc.subject
BaTaO2N  
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Crystal structure  
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Oxynitride  
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Photocatalysis  
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Synthesis  
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Water splitting  
dc.subject.classification
Físico-Química, Ciencia de los Polímeros, Electroquímica  
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Ciencias Químicas  
dc.subject.classification
CIENCIAS NATURALES Y EXACTAS  
dc.title
Perovskite BaTaO 2 N: From Materials Synthesis to Solar Water Splitting  
dc.type
info:eu-repo/semantics/article  
dc.type
info:ar-repo/semantics/artículo  
dc.type
info:eu-repo/semantics/publishedVersion  
dc.date.updated
2024-11-26T11:24:16Z  
dc.journal.volume
10  
dc.journal.number
33  
dc.journal.pagination
1-47  
dc.journal.pais
Estados Unidos  
dc.description.fil
Fil: Hojamberdiev, Mirabbos. Technische Universität Berlin; Alemania  
dc.description.fil
Fil: Vargas Balda, Ronald Eduardo. Consejo Nacional de Investigaciones Científicas y Técnicas. Centro Científico Tecnológico Conicet - La Plata. Instituto de Investigaciones Biotecnológicas. Universidad Nacional de San Martín. Instituto de Investigaciones Biotecnológicas; Argentina  
dc.description.fil
Fil: Zhang, Fuxiang. Chinese Academy of Sciences; República de China  
dc.description.fil
Fil: Teshima, Katsuya. Shinshu University; Alemania  
dc.description.fil
Fil: Lerch, Martin. Technische Universität Berlin; Alemania  
dc.journal.title
Advanced Science  
dc.relation.alternativeid
info:eu-repo/semantics/altIdentifier/url/https://onlinelibrary.wiley.com/doi/10.1002/advs.202305179  
dc.relation.alternativeid
info:eu-repo/semantics/altIdentifier/doi/http://dx.doi.org/10.1002/advs.202305179