Artículo
Effective treatment of charge and spin fluctuations in dynamical and static atom-surface interactions
Fecha de publicación:
12/2009
Editorial:
American Physical Society
Revista:
Physical Review B: Condensed Matter and Materials Physics
ISSN:
1098-0121
Idioma:
Inglés
Tipo de recurso:
Artículo publicado
Clasificación temática:
Resumen
In this work we introduce a formalism that provides a good description of the correlated charge states of an atom interacting statically or dynamically with a metal surface, including realistic features of the atom-surface system. Our treatment of the Anderson impurity with an intrasite finite repulsion is based on the use of a projection operator technique and the application of the equation of motion method. The specific case of charge state configurations having zero, one, and two valence electrons of atoms with s-type valence orbital is discussed in this work. Static properties, such as the average occupation and the local density of states at the atom site and dynamical charge fractions in atom scattering processes, are compared with exact calculations and also with other existing approximations. Our treatment of the finite electronic repulsion at the atom site also reproduces satisfactorily the experimental behavior of the transmission phase shift of a dot measured by Aharonov-Bohm interferometry in both weak and strong coupling limits.
Palabras clave:
Charge And Spin Fluctuations
,
Strong Correlated Electrons
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Articulos(INTEC)
Articulos de INST.DE DES.TECNOL.PARA LA IND.QUIMICA (I)
Articulos de INST.DE DES.TECNOL.PARA LA IND.QUIMICA (I)
Citación
Romero, Marcelo Ariel; Flores, F.; Goldberg, Edith Catalina; Effective treatment of charge and spin fluctuations in dynamical and static atom-surface interactions; American Physical Society; Physical Review B: Condensed Matter and Materials Physics; 80; 23; 12-2009; 1-13; 235427
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