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dc.contributor.author
Alas, S. J.
dc.contributor.author
Rojas, F.
dc.contributor.author
Kornhauser, I.
dc.contributor.author
Zgrablich, Jorge Andres
dc.date.available
2022-05-27T12:44:33Z
dc.date.issued
2006-02
dc.identifier.citation
Alas, S. J.; Rojas, F.; Kornhauser, I.; Zgrablich, Jorge Andres; Dynamic Monte Carlo simulation of oscillations and pattern formation during the NO+CO reaction on the Pt (100) surface; Elsevier Science; Journal of Molecular Catalysis A: Chemical; 244; 1-2; 2-2006; 183-192
dc.identifier.issn
1381-1169
dc.identifier.uri
http://hdl.handle.net/11336/158336
dc.description.abstract
Theoretical simulations by a dynamic Monte Carlo method were carried out with respect to the catalytic reduction of NO by CO on the Pt(100) surface. This reaction, when occurring at low pressures and under certain reaction conditions, exhibits different temporal and spatiotemporal behaviors, caused by an adsorbate-induced surface restructuring. The studies herein developed take into account recent experimental evidences concerning the NO+CO reaction on the Rh(111) surface; such experiments have shown that the production of molecular nitrogen occurs preferentially via the formation of an (N–NO)* intermediary species rather than through the conventional N+N recombination step. Sustained, irregular or damped oscillations as well as the formation of cellular structures and turbulent patterns are observed during our Monte Carlo surface reaction analysis.
dc.format
application/pdf
dc.language.iso
eng
dc.publisher
Elsevier Science
dc.rights
info:eu-repo/semantics/openAccess
dc.rights.uri
https://creativecommons.org/licenses/by-nc-sa/2.5/ar/
dc.subject
NO REDUCTION
dc.subject
KINETIC OSCILLATIONS
dc.subject
REACTION PATTERN FORMATION
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SURFACE RECONSTRUCTION
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DYNAMIC MONTE CARLO SIMULATION
dc.subject.classification
Otras Ciencias Químicas
dc.subject.classification
Ciencias Químicas
dc.subject.classification
CIENCIAS NATURALES Y EXACTAS
dc.title
Dynamic Monte Carlo simulation of oscillations and pattern formation during the NO+CO reaction on the Pt (100) surface
dc.type
info:eu-repo/semantics/article
dc.type
info:ar-repo/semantics/artículo
dc.type
info:eu-repo/semantics/publishedVersion
dc.date.updated
2022-05-20T15:07:51Z
dc.journal.volume
244
dc.journal.number
1-2
dc.journal.pagination
183-192
dc.journal.pais
Países Bajos
dc.journal.ciudad
Amsterdam
dc.description.fil
Fil: Alas, S. J.. Universidad Autónoma Metropolitana; México
dc.description.fil
Fil: Rojas, F.. Universidad Autónoma Metropolitana; México
dc.description.fil
Fil: Kornhauser, I.. Universidad Autónoma Metropolitana; México
dc.description.fil
Fil: Zgrablich, Jorge Andres. Consejo Nacional de Investigaciones Científicas y Técnicas. Centro Científico Tecnológico Conicet - San Luis; Argentina. Universidad Nacional de San Luis. Facultad de Ciencias Fisico Matematicas y Naturales. Departamento de Fisica. Laboratorio de Ciencias de Superficies y Medios Porosos; Argentina
dc.journal.title
Journal of Molecular Catalysis A: Chemical
dc.relation.alternativeid
info:eu-repo/semantics/altIdentifier/url/https://www.sciencedirect.com/science/article/abs/pii/S1381116905006801
dc.relation.alternativeid
info:eu-repo/semantics/altIdentifier/doi/https://doi.org/10.1016/j.molcata.2005.09.029
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