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dc.contributor.author
Souza, Thiago Leandro de
dc.contributor.author
Rossi, Carla Cassia Rodrigues Da Silva
dc.contributor.author
Alonso, Christian Gonçalves
dc.contributor.author
Guirardello, Reginaldo
dc.contributor.author
Cabral, Vladimir Ferreira
dc.contributor.author
Fernandes Machado, Nádia Regina Camargo
dc.contributor.author
Specchia, Stefania
dc.contributor.author
Zabaloy, Marcelo Santiago
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dc.contributor.author
Cardozo Filho, Lucio
dc.date.available
2017-04-17T18:32:00Z
dc.date.issued
2013-10
dc.identifier.citation
Souza, Thiago Leandro de; Rossi, Carla Cassia Rodrigues Da Silva; Alonso, Christian Gonçalves; Guirardello, Reginaldo; Cabral, Vladimir Ferreira; et al.; Thermodynamic analysis of autothermal reforming of methane via entropy maximization: Hydrogen production; Elsevier; International Journal Of Hydrogen Energy; 39; 16; 10-2013; 8257-8270
dc.identifier.issn
0360-3199
dc.identifier.uri
http://hdl.handle.net/11336/15315
dc.description.abstract
In this work a thermodynamic analysis of the autothermal reforming (ATR) of methane was performed. Equilibrium calculations employing entropy maximization were performed in a wide range of oxygen to methane mole ratio (O/M), steam to methane ratio (S/ M), inlet temperature (IT), and system pressure (P). The main calculated parameters were hydrogen yield, carbon monoxide formation, methane conversion, coke formation, and equilibrium temperature. Further, the optimum operating oxygen to methane feed ratio that maximizes hydrogen production, at P ¼ 1 bar, has been calculated. The nonlinear programming problem applied to the simultaneous chemical and phase equilibrium calculation was implemented in GAMS, using CONOPT2 solver. The maximum amount of hydrogen obtained was in the order of 3 moles of hydrogen per mole of fed methane at IT ¼ 1000 C, P ¼ 1 bar, S/M ¼ 5, and O/M ¼ 0.18. Experimental literature data are in good agreement with calculation results obtained through proposed methodology.
dc.format
application/pdf
dc.language.iso
eng
dc.publisher
Elsevier
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dc.rights
info:eu-repo/semantics/openAccess
dc.rights.uri
https://creativecommons.org/licenses/by-nc-nd/2.5/ar/
dc.subject
Methane Autothermal Reforming
dc.subject
Hydrogen
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Entropy Maximization
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Optimization
dc.subject.classification
Otras Ingeniería Química
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dc.subject.classification
Ingeniería Química
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dc.subject.classification
INGENIERÍAS Y TECNOLOGÍAS
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dc.title
Thermodynamic analysis of autothermal reforming of methane via entropy maximization: Hydrogen production
dc.type
info:eu-repo/semantics/article
dc.type
info:ar-repo/semantics/artículo
dc.type
info:eu-repo/semantics/publishedVersion
dc.date.updated
2015-06-24T20:21:22Z
dc.journal.volume
39
dc.journal.number
16
dc.journal.pagination
8257-8270
dc.journal.pais
Países Bajos
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dc.journal.ciudad
Amsterdam
dc.description.fil
Fil: Souza, Thiago Leandro de. Universidade Estadual de Maringá; Brasil
dc.description.fil
Fil: Rossi, Carla Cassia Rodrigues Da Silva. Universidade Estadual de Campinas; Brasil
dc.description.fil
Fil: Alonso, Christian Gonçalves. Universidade Federal de Goias; Brasil
dc.description.fil
Fil: Guirardello, Reginaldo. Universidade Estadual de Campinas; Brasil
dc.description.fil
Fil: Cabral, Vladimir Ferreira. Universidade Estadual de Maringá; Brasil
dc.description.fil
Fil: Fernandes Machado, Nádia Regina Camargo. Universidade Estadual de Maringá; Brasil
dc.description.fil
Fil: Specchia, Stefania. Politecnico Di Torino; Italia
dc.description.fil
Fil: Zabaloy, Marcelo Santiago. Consejo Nacional de Investigaciones Científicas y Técnicas. Centro Científico Tecnológico Bahía Blanca. Planta Piloto de Ingeniería Química (i); Argentina; Argentina. Universidad Nacional del Sur; Argentina
dc.description.fil
Fil: Cardozo Filho, Lucio. Universidade Estadual de Maringá; Brasil
dc.journal.title
International Journal Of Hydrogen Energy
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dc.relation.alternativeid
info:eu-repo/semantics/altIdentifier/doi/http://dx.doi.org/10.1016/j.ijhydene.2014.03.078
dc.relation.alternativeid
info:eu-repo/semantics/altIdentifier/url/http://www.sciencedirect.com/science/article/pii/S0360319914007344
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