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dc.contributor.author
Rodriguez, Maria Laura
dc.contributor.author
Cadus, Luis Eduardo
dc.date.available
2017-04-05T15:05:05Z
dc.date.issued
2015-12
dc.identifier.citation
Rodriguez, Maria Laura; Cadus, Luis Eduardo; Mass transfer limitations in a monolithic reactor for the catalytic oxidation of ethanol; Elsevier; Chemical Engineering Science; 143; 12-2015; 305-313
dc.identifier.issn
0009-2509
dc.identifier.uri
http://hdl.handle.net/11336/14826
dc.description.abstract
A theoretical study of a monolithic reactor for the catalytic oxidation of Volatile Organic Compounds (VOC) over manganese–copper mixed oxide catalysts is presented. An isothermal one-dimensional heterogeneous model is selected to account for the external (gas–solid) and internal (washcoat) mass transport limitations.
The results reveal that under certain operating conditions, e.g. thick washcoats and high conversions of VOCs (high temperatures), the overall process rate is reduced by internal diffusion inside the catalyst. At high temperatures and/or monoliths with poor interfacial areas, the overall process rate is limited by external mass transfer resistance to the catalyst. Proper quantification of both internal and external mass transfer resistances by means of a heterogeneous model can result in avoiding situations of incomplete VOC abatement under conditions of high VOC dilution.
dc.format
application/pdf
dc.language.iso
eng
dc.publisher
Elsevier
dc.rights
info:eu-repo/semantics/openAccess
dc.rights.uri
https://creativecommons.org/licenses/by-nc-sa/2.5/ar/
dc.subject
Catalytic Oxidation
dc.subject
Monolithic Reactor
dc.subject
Heterogeneous Model
dc.subject
Mass Transfer
dc.subject
Ethanol
dc.subject.classification
Otras Ingeniería Química
dc.subject.classification
Ingeniería Química
dc.subject.classification
INGENIERÍAS Y TECNOLOGÍAS
dc.title
Mass transfer limitations in a monolithic reactor for the catalytic oxidation of ethanol
dc.type
info:eu-repo/semantics/article
dc.type
info:ar-repo/semantics/artículo
dc.type
info:eu-repo/semantics/publishedVersion
dc.date.updated
2017-03-31T18:25:27Z
dc.journal.volume
143
dc.journal.pagination
305-313
dc.journal.pais
Países Bajos
dc.journal.ciudad
Amsterdam
dc.description.fil
Fil: Rodriguez, Maria Laura. Consejo Nacional de Investigaciones Científicas y Técnicas. Centro Científico Tecnológico San Luis. Instituto de Investigaciones en Tecnología Química; Argentina
dc.description.fil
Fil: Cadus, Luis Eduardo. Consejo Nacional de Investigaciones Científicas y Técnicas. Centro Científico Tecnológico San Luis. Instituto de Investigaciones en Tecnología Química; Argentina
dc.journal.title
Chemical Engineering Science
dc.relation.alternativeid
info:eu-repo/semantics/altIdentifier/url/http://www.sciencedirect.com/science/article/pii/S0009250915007873
dc.relation.alternativeid
info:eu-repo/semantics/altIdentifier/doi/http://dx.doi.org/10.1016/j.ces.2015.12.010
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