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dc.contributor.author
De La Cruz Félix, Nelphy
dc.contributor.author
Centres, Paulo Marcelo
dc.contributor.author
Ramirez Pastor, Antonio Jose
dc.contributor.author
Vogel, Eugenio Emilio
dc.contributor.author
Valdés, Julio Félix
dc.date.available
2021-07-20T21:47:32Z
dc.date.issued
2020-07
dc.identifier.citation
De La Cruz Félix, Nelphy; Centres, Paulo Marcelo; Ramirez Pastor, Antonio Jose; Vogel, Eugenio Emilio; Valdés, Julio Félix; Irreversible multilayer adsorption of semirigid k -mers deposited on one-dimensional lattices; American Physical Society; Physical Review E: Statistical, Nonlinear and Soft Matter Physics; 102; 1; 7-2020; 1-11; 012106
dc.identifier.issn
2470-0045
dc.identifier.uri
http://hdl.handle.net/11336/136536
dc.description.abstract
Irreversible multilayer adsorption of semirigid k -mers on one-dimensional lattices of size L is studied by numerical simulations complemented by exhaustive enumeration of configurations for small lattices. The deposition process is modeled by using a random sequential adsorption algorithm, generalized to the case of multilayer adsorption. The paper concentrates on measuring the jamming coverage for different values of k -mer size and number of layers n . The bilayer problem ( n ≤ 2 ) is exhaustively analyzed, and the resulting tendencies are validated by the exact enumeration techniques. Then, the study is extended to an increasing number of layers, which is one of the noteworthy parts of this work. The obtained results allow the following: (i) to characterize the structure of the adsorbed phase for the multilayer problem. As n increases, the ( 1 + 1 ) -dimensional adsorbed phase tends to be a “partial wall” consisting of “towers” (or columns) of width k , separated by valleys of empty sites. The length of these valleys diminishes with increasing k ; (ii) to establish that this is an in-registry adsorption process, where each incoming k -mer is likely to be adsorbed exactly onto an already adsorbed one. With respect to percolation, our calculations show that the percolation probability vanishes as L increases, being zero in the limit L → ∞ . Finally, the value of the jamming critical exponent ν j is reported here for multilayer adsorption: ν j remains close to 2 regardless of the considered values of k and n . This finding is discussed in terms of the lattice dimensionality.
dc.format
application/pdf
dc.language.iso
eng
dc.publisher
American Physical Society
dc.rights
info:eu-repo/semantics/openAccess
dc.rights.uri
https://creativecommons.org/licenses/by-nc-sa/2.5/ar/
dc.subject
JAMMING
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PERCOLATION
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SEMIIRIGID
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K-MERS
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Otras Ciencias Físicas
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Ciencias Físicas
dc.subject.classification
CIENCIAS NATURALES Y EXACTAS
dc.title
Irreversible multilayer adsorption of semirigid k -mers deposited on one-dimensional lattices
dc.type
info:eu-repo/semantics/article
dc.type
info:ar-repo/semantics/artículo
dc.type
info:eu-repo/semantics/publishedVersion
dc.date.updated
2021-04-22T20:45:53Z
dc.identifier.eissn
2470-0053
dc.journal.volume
102
dc.journal.number
1
dc.journal.pagination
1-11; 012106
dc.journal.pais
Estados Unidos
dc.description.fil
Fil: De La Cruz Félix, Nelphy. Universidad Nacional de San Luis; Argentina. Universidad Autonoma de Santo Domingo.; República Dominicana
dc.description.fil
Fil: Centres, Paulo Marcelo. Consejo Nacional de Investigaciones Científicas y Técnicas. Centro Científico Tecnológico Conicet - San Luis. Instituto de Física Aplicada "Dr. Jorge Andrés Zgrablich". Universidad Nacional de San Luis. Facultad de Ciencias Físico Matemáticas y Naturales. Instituto de Física Aplicada "Dr. Jorge Andrés Zgrablich"; Argentina
dc.description.fil
Fil: Ramirez Pastor, Antonio Jose. Consejo Nacional de Investigaciones Científicas y Técnicas. Centro Científico Tecnológico Conicet - San Luis. Instituto de Física Aplicada "Dr. Jorge Andrés Zgrablich". Universidad Nacional de San Luis. Facultad de Ciencias Físico Matemáticas y Naturales. Instituto de Física Aplicada "Dr. Jorge Andrés Zgrablich"; Argentina
dc.description.fil
Fil: Vogel, Eugenio Emilio. Universidad de La Frontera; Chile. Center for the Development of Nanoscience and Nanotechnology; Chile
dc.description.fil
Fil: Valdés, Julio Félix. Universidad de La Frontera; Chile
dc.journal.title
Physical Review E: Statistical, Nonlinear and Soft Matter Physics
dc.relation.alternativeid
info:eu-repo/semantics/altIdentifier/doi/http://dx.doi.org/10.1103/PhysRevE.102.012106
dc.relation.alternativeid
info:eu-repo/semantics/altIdentifier/url/https://journals.aps.org/pre/abstract/10.1103/PhysRevE.102.012106
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