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dc.contributor.author
Soria Castro, Silvia Mercedes
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dc.contributor.author
Lebeau, Benedicte
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dc.contributor.author
Cormier, Morgan
dc.contributor.author
Neunlist, Serge
dc.contributor.author
Daou, T. Jean
dc.contributor.author
Goddard, Jean-Philippe
dc.date.available
2020-12-09T20:15:11Z
dc.date.issued
2020-03
dc.identifier.citation
Soria Castro, Silvia Mercedes; Lebeau, Benedicte; Cormier, Morgan; Neunlist, Serge; Daou, T. Jean; et al.; Organic/Inorganic heterogeneous silica-based photoredox catalyst for Aza-Henry Reactions; Wiley VCH Verlag; European Journal of Organic Chemistry; 2020; 10; 3-2020; 1572-1578
dc.identifier.issn
1434-193X
dc.identifier.uri
http://hdl.handle.net/11336/120039
dc.description.abstract
The transformation of light into chemical energy is a leitmotiv in the development of sustainable and environmentally concerned chemical processes. Chemists invented original concepts to address this purpose, like photoredox catalysis, which became a wonderful tool to transform simple organic compounds into high-value products. Nevertheless, the most relevant transition metal based photocatalysts suffer from major disadvantages like toxicity, cost, and poor recyclability potential. To circumvent this, we propose a new generation of heterogeneous photoredox catalysts resulting from the combination of porous silica materials and Rose Bengal. They promote carbon–carbon bond formations under visible-light in environmentally benign solvent using air as the only stoichiometric redox partner. The pure covalent photocatalytic system provides a robust and recyclable system for greener catalysis. This report would be of broad significance because it addresses important sustainability issues: recycling, non-toxic metal-free photocatalysts, and less-waste-producing chemical process.
dc.format
application/pdf
dc.language.iso
eng
dc.publisher
Wiley VCH Verlag
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dc.rights
info:eu-repo/semantics/restrictedAccess
dc.rights.uri
https://creativecommons.org/licenses/by-nc-sa/2.5/ar/
dc.subject
HETEROGENEOUS CATALYSIS
dc.subject
ORDERED MESOPOROUS SILICA
dc.subject
PHOTOREDOX CATALYSIS
dc.subject
SYNTHETIC METHODS
dc.subject
ZEOLITES
dc.subject.classification
Química Orgánica
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dc.subject.classification
Ciencias Químicas
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dc.subject.classification
CIENCIAS NATURALES Y EXACTAS
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dc.title
Organic/Inorganic heterogeneous silica-based photoredox catalyst for Aza-Henry Reactions
dc.type
info:eu-repo/semantics/article
dc.type
info:ar-repo/semantics/artículo
dc.type
info:eu-repo/semantics/publishedVersion
dc.date.updated
2020-11-17T18:34:28Z
dc.identifier.eissn
1099-0690
dc.journal.volume
2020
dc.journal.number
10
dc.journal.pagination
1572-1578
dc.journal.pais
Alemania
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dc.journal.ciudad
Weinheim
dc.description.fil
Fil: Soria Castro, Silvia Mercedes. Université de Strasbourg; Francia. Université Haute-alsace. Institut de Science Des Matériaux de Mulhouse.; Francia
dc.description.fil
Fil: Lebeau, Benedicte. Université de Strasbourg; Francia. Université Haute-alsace. Institut de Science Des Matériaux de Mulhouse.; Francia
dc.description.fil
Fil: Cormier, Morgan. Université Haute-alsace.; Francia
dc.description.fil
Fil: Neunlist, Serge. Université Haute-alsace.; Francia
dc.description.fil
Fil: Daou, T. Jean. Université de Strasbourg; Francia
dc.description.fil
Fil: Goddard, Jean-Philippe. Université Haute-alsace.; Francia
dc.journal.title
European Journal of Organic Chemistry
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dc.relation.alternativeid
info:eu-repo/semantics/altIdentifier/url/http://doi.wiley.com/10.1002/ejoc.201901382
dc.relation.alternativeid
info:eu-repo/semantics/altIdentifier/doi/http://dx.doi.org/10.1002/ejoc.201901382
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