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Artículo

Semiempirical model for analysis of inhomogeneous optically thick laser-induced plasmas

D'angelo, Cristian Adrián; Diaz Pace, Diego MartinIcon ; Bertuccelli, GracielaIcon
Fecha de publicación: 10/2009
Editorial: Pergamon-Elsevier Science Ltd
Revista: Spectrochimica Acta Part B: Atomic Spectroscopy
ISSN: 0584-8547
Idioma: Inglés
Tipo de recurso: Artículo publicado
Clasificación temática:
Física Atómica, Molecular y Química

Resumen

Abstract In this paper, a more realistic approach of a non-uniform optically thick plasma in local thermodynamic equilibrium was applied to describe self-reversal of Co I 340.51 nm emission line recorded from a laser-induced plasma generated on a Co Cr Mo metallic alloy. This line was selected because it is one of the most absorbed of the major elements in air at atmospheric pressure. The model describes the behavior of the plasma after the breakdown, and it was semiempirical thus, some information was taken from the experiment. A cylinder-symmetrical plasma column with a parabolic temperature distribution having a maximum at the center and decreasing toward the edges was considered. The input parameters were the plasma length, the temperature in the plasma core, and the Co total density, which were estimated from measurements and previous work. Moreover, the distribution of electron density depended on the temperature, and the ionization degree was taken into account through Saha equation. Then, plasma parameters were adjusted in such a way calculations reproduced the experimentally measured line profiles. The effect of varying laser power on plasma homogeneity and its evolution in time were investigated. Moreover, preliminary results of spatial distribution of plasma parameters were obtained that confirmed the practical application of the model on plasma diagnostics.
Palabras clave: LIBS , Optically thick plasma , Inhomogeneous plasma , Metallic alloys
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info:eu-repo/semantics/openAccess Excepto donde se diga explícitamente, este item se publica bajo la siguiente descripción: Creative Commons Attribution-NonCommercial-ShareAlike 2.5 Unported (CC BY-NC-SA 2.5)
Identificadores
URI: http://hdl.handle.net/11336/111770
URL: http://www.sciencedirect.com/science/article/pii/S0584854709001980
Colecciones
Articulos(CCT - TANDIL)
Articulos de CTRO CIENTIFICO TECNOLOGICO CONICET - TANDIL
Articulos(CIFICEN)
Articulos de CENTRO DE INV. EN FISICA E INGENIERIA DEL CENTRO DE LA PCIA. DE BS. AS.
Citación
D'angelo, Cristian Adrián; Diaz Pace, Diego Martin; Bertuccelli, Graciela; Semiempirical model for analysis of inhomogeneous optically thick laser-induced plasmas; Pergamon-Elsevier Science Ltd; Spectrochimica Acta Part B: Atomic Spectroscopy; 64; 10; 10-2009; 999-1008
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