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dc.contributor.author
Cencha, Luisa Guadalupe
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Huber, Patrick
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Kappl, Michael
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Floudas, George
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Steinhart, Martin
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Berli, Claudio Luis Alberto
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Urteaga, Raul
dc.date.available
2020-06-07T21:52:49Z
dc.date.issued
2019-09
dc.identifier.citation
Cencha, Luisa Guadalupe; Huber, Patrick; Kappl, Michael; Floudas, George; Steinhart, Martin; et al.; Nondestructive high-throughput screening of nanopore geometry in porous membranes by imbibition; American Institute of Physics; Applied Physics Letters; 115; 11; 9-2019; 113701-1/5
dc.identifier.issn
0003-6951
dc.identifier.uri
http://hdl.handle.net/11336/106815
dc.description.abstract
A fluid dynamic model for imbibition into closed-end, axisymmetric pores having diameters that change as a function of the pore depth is presented. Despite the fact that liquid invasion into nonbranched closed-end pores is characterized by a wealth of different transient and/or metastable nonequilibrium stages related to precursor film formation, we show that a simple hydraulic model accounting for geometry- and air compression-induced deviations from classical Lucas-Washburn dynamics precisely describes the imbibition dynamics except at the late stage. The model was validated by laser interferometry experiments with submillisecond temporal resolution. Imbibition of three simple liquids (isopropanol, ethanol, and hexane) into self-ordered anodic alumina membranes containing arrays of parallel closed-end nanopores characterized by slight conicity was studied. The model provides an improved description of nanoscale fluid dynamics and allows geometric characterization of nanoporous membranes by their imbibition kinetics accounting for the back pressure of the compressed gas. Thus, a precise calibration of porous membranes with simple liquids becomes possible, and changes in the mean pore diameter as a function of the pore depth can be assessed.
dc.format
application/pdf
dc.language.iso
eng
dc.publisher
American Institute of Physics
dc.rights
info:eu-repo/semantics/embargoedAccess
dc.rights.uri
https://creativecommons.org/licenses/by-nc-sa/2.5/ar/
dc.subject
Nanochannels
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Capillary imbibition
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Microfluidics
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Optofluidic model
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Otras Nanotecnología
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Nanotecnología
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INGENIERÍAS Y TECNOLOGÍAS
dc.title
Nondestructive high-throughput screening of nanopore geometry in porous membranes by imbibition
dc.type
info:eu-repo/semantics/article
dc.type
info:ar-repo/semantics/artículo
dc.type
info:eu-repo/semantics/publishedVersion
dc.date.updated
2020-06-01T13:36:45Z
dc.journal.volume
115
dc.journal.number
11
dc.journal.pagination
113701-1/5
dc.journal.pais
Estados Unidos
dc.description.fil
Fil: Cencha, Luisa Guadalupe. Consejo Nacional de Investigaciones Científicas y Técnicas. Centro Científico Tecnológico Conicet - Santa Fe. Instituto de Física del Litoral. Universidad Nacional del Litoral. Instituto de Física del Litoral; Argentina
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Fil: Huber, Patrick. Hamburg University Of Technology;
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Fil: Kappl, Michael. Max-planck-institut Für Polymerforschung;
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Fil: Floudas, George. Panepistimion Ioanninon;
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Fil: Steinhart, Martin. Max-planck-institut Für Polymerforschung;
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Fil: Berli, Claudio Luis Alberto. Consejo Nacional de Investigaciones Científicas y Técnicas. Centro Científico Tecnológico Conicet - Santa Fe. Instituto de Desarrollo Tecnológico para la Industria Química. Universidad Nacional del Litoral. Instituto de Desarrollo Tecnológico para la Industria Química; Argentina
dc.description.fil
Fil: Urteaga, Raul. Consejo Nacional de Investigaciones Científicas y Técnicas. Centro Científico Tecnológico Conicet - Santa Fe. Instituto de Física del Litoral. Universidad Nacional del Litoral. Instituto de Física del Litoral; Argentina
dc.journal.title
Applied Physics Letters
dc.rights.embargoDate
2020-09-10
dc.relation.alternativeid
info:eu-repo/semantics/altIdentifier/doi/https://doi.org/10.1063/1.5119338
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